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Quantum Optics VI: Laser Cooling

Blogs > Ideal26
Post a Reply
Ideal26
Profile Blog Joined November 2013
United States185 Posts
June 01 2014 14:40 GMT
#1
Hey again!

I think we struck gold with last week's topic, and I just have to thank you all for such stimulating conversations! I learned so much in attempts to answer your questions and by reading other’s answers and I hope you guys learned something too. I might fall back to that post for inspiration for future blog topics, as a lot of really deep questions were asked that are just begging for more attention.

I already had a draft prepared for this week, however, so I’m going to stick with it. It’s a pretty cute and common technique now, but you might not know much about it if you haven’t played around in an atomic physics lab before.


Lesson 6: Laser Cooling

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Scientists have been extremely interested in performing experiments at ultra-low temperatures. If you can isolate and almost freeze an atom in its tracks, it becomes much easier for you to probe the atom and investigate its structure. You can also observe a lot of crazy quantum effects, like Bose-Einstein condensation, superfluidity, etc. We’ll probably talk about those things in the future.

There are several variations on the theme of laser/atomic cooling these days, but we’re going to start with the simplest and most common method: Doppler cooling.


Say you have a little cloud of atoms; a gas of some particular element. We know by now that atoms can absorb/emit photons of certain discrete energies, right? We shine a laser (say the beam is traveling to the left, for example) of a frequency that is slightly red-shifted from an allowed atomic energy transitions. Any atom that is just sitting still will see a photon with a wavelength that is too long, so it can’t absorb the light. This is where the word Doppler comes in.


The atoms in our cloud aren’t stationary; they have some nonzero velocity. These atoms see frequencies that are Doppler shifted up or down by an amount:

+ Show Spoiler +
∆f=(V/c) f_laser

V=velocity of atom, c= speed of light, f_laser is the laser frequency


An atom that is moving to the left, with the beam, will see an even further red shifted beam and it won’t absorb the photons. An atom moving to the right (at the correct velocity), however, will see a photon with just the right energy for absorption. Note that there is a bit of "bandwidth" for the absorption probability; it isn't huge, but the velocities don't have to be so exactly perfect that the probability of absorption is almost zero.


+ Show Spoiler +

[image loading]
A. A stationary atom "sees" light with a wavelength that is too long for it to absorb.
B. An atom moving in the same direction as the beam sees a wavelength that is too long, and also will not absorb a photon.
C. An atom moving toward the beam sees a shorter wavelength that is resonant with the atomic transition, and absorbs a photon.

(disclaimer because some people take over-simplifications too much to heart; the colors are of course exaggerated, the frequency shifts are not so huge that the wavelength changes by hundreds of nm, its just for illustrative purposes)



The atom absorbs the photon and its associated momentum (which was in the opposite direction to the atom’s direction) and the atom slows down a little. The atom is now in an excited state though, because of this extra energy, and it’ll emit a photon in return. If the photon beam is weak enough, emission is usually spontaneous (there aren’t enough photons around to stimulate emission in many of the atoms). Spontaneous emission, if you recall, is when the atom emits the photon in a random direction. When this happens to the atom in our cloud, it’ll receive a momentum kick.


+ Show Spoiler +
[image loading]



The net result of this interaction is that the atom originally moving right with a high velocity has been slowed down and redirected, if only by a little bit. In a real cloud of atoms with real lasers, these interactions will happen frequently and the atoms will slow down to very low speeds rapidly.

Of course, as the atoms slow down, they no longer “see” the appropriate frequency of light and cannot continuously absorb photons, so the frequency of the laser must be adjusted.
An alternative to frequency sweeping is something called “Zeeman slowing” (related to the Zeeman effect) that uses magnetic fields. Simply put, the application of a magnetic field to an atom causes changes in its resonance frequency- the frequency of photon it’ll readily absorb.


We want to slow our atoms in all directions though, not just slow the ones moving to the right. To accomplish this we simply add a laser traveling in the opposite direction. Extending this idea, 3 perpendicular sets of oppositely directed beams would allow us to slow atoms in all directions, creating a cloud of low-velocity, and therefore low kinetic energy, atoms. The relationship between kinetic energy and temperature is where the term “cooling” came from, and so we often report how slow we can get the atoms in units of temperature. This sort of cooling set up alone gets us down to the hundreds of mili-Kelvin range.

When you use counter-propagating circularly polarized beams in this configuration, you can create what the call “optical molasses”. Without going into too many details, the appropriately polarized laser beams create a polarization gradient (a change in the polarization with location) and the atoms lose energy as they climb “up” the gradient. This sort of acts like a viscous drag force, hence the name “molasses”.


Laser cooling is often coupled with magnetic trapping, creating a “magneto-optical trap”, or a MOT. A magnetic field is set up to so that when an atom approaches the edges of the “trap” it is redirected back toward the center.

+ Show Spoiler +
[image loading]


+ Show Spoiler +
[image loading]
An actual MOT with Ytterbium atoms.
Image from: http://www.quantum-munich.de/research/ytterbium-quantum-gases-in-optical-lattices/



Doppler cooling is limited, as eventually the atoms become so slow that absorbing/re-emitting photons actually increases their energy as often as it decreases their energy. The lower bound on the temperature we can achieve using this simple idea is appropriately called the Doppler limit.
The use of polarization gradients to overcome this limit is very common, as is evaporative cooling.
It’s not uncommon to see all of these things combined; start by slowing the atoms considerably using Doppler cooling, load them into a MOT and further cool them by applying particular magnetic fields or polarization gradients. These sort of setups have achieved temperatures on the order of micro-Kelvin.

We should also note that not all atoms can be laser cooled by Doppler cooling; they have to have an energy level structure that works with the lasers (=photon energies) we have available.


This was an extremely short entry compared to my others, so for entertainment and because it’s relevant, pictures! Once upon a time I built a laser for an atomic physics lab, and now it’s being used for laser cooling experiments. It was a terribly tedious project, but finally getting it to lase correctly was the best feeling ever. They aren't high quality or that interesting of photos, but this was the first laser system I ever made and I just adore it.


+ Show Spoiler +

[image loading]
This is the majority of the main laser setup, except a few things were changed after this photo was taken... nothing important though, just re-arranging and the addition of a lens. If you're familiar with lasers, this is actually a slave in a master/slave system. It's coupled via the fiber you see on the left to the master in another lab a few rooms over, which is where the rest of my set up is. If you want more details on master/slave lasers, just ask.


+ Show Spoiler +

[image loading]
This includes the diagnostic equipment used to get everything running right.


+ Show Spoiler +

[image loading]
Anddd with the lights dimmed, so you can see that yes, it is actually producing light. Of the correct wavelength, even!




Thanks for reading! As always, I really, really appreciate your questions and feedback, good or bad!
Your responses always make these blogs so much fun to post. <3

*****
airen
Profile Joined September 2004
Sweden82 Posts
June 01 2014 18:51 GMT
#2
Very nice, I've heard of cooling with lasers, but never had any insight into how it's done. Explanation was very easy to understand.

Not knowing much about optics, and looking at your pictures, how much of a disturbance is regular air to conducting experiments? I've always kind of figured that all such experiments were done in vacuum, but looking at your pictures (and recalling others) this never seem to be the case?
urboss
Profile Joined September 2013
Austria1223 Posts
June 01 2014 19:39 GMT
#3
Cool stuff; I have some questions:
- Is the time between absorption and emission always the same?
- Can this be done with molecules as well?
- Can the same technique be used to accelerate atoms (why would you wanna do that)?
Ideal26
Profile Blog Joined November 2013
United States185 Posts
June 01 2014 20:39 GMT
#4
On June 02 2014 03:51 airen wrote:
Not knowing much about optics, and looking at your pictures, how much of a disturbance is regular air to conducting experiments? I've always kind of figured that all such experiments were done in vacuum, but looking at your pictures (and recalling others) this never seem to be the case?

The chamber in which the atoms to be cooled are located will be in vacuum (the photo of the MOT shows the atom cloud in a vacuum chamber). The actual laser though, that doesn’t have to be in vacuum conditions. The refractive index of air is extremely close to 1, so light travels through air pretty much the same way it travels through vacuum. Air doesn't complicate laser setups nearly as much as things like imperfect lenses and mirrors do.

On June 02 2014 04:39 urboss wrote:
Cool stuff; I have some questions:
- Is the time between absorption and emission always the same?
- Can this be done with molecules as well?
- Can the same technique be used to accelerate atoms (why would you wanna do that)?


1. The rate of spontaneous emission depends on both the atom and the surrounding field. The rate of decay is exponential; decays have the form exp(-t/T) where T is the “lifetime” of the atom. This means that half of the atoms decay after t=ln(2)= 0.693ish. So the time between absorption and emission isn't exactly fixed; as is common with quantum phenomena it follows a sort of probability distribution.

2. Not really.. It can only be done with select atoms because of the requirements on the resonance conditions, and molecules are just too complicated when it comes to resonance frequencies. There are a view papers out there that illustrate cooling diatomic molecules, but this isn't something that’s easily reproducible or developed well enough to be useful.

3. My instinct told me “well sure, why not?” but I hadn't heard of doing such a thing, so I looked it up. Apparently they use lasers for something called “plasma acceleration”. The idea is quite different though- it isn't absorption/emission related. They basically bombard atoms with ultrashort laser pulses and strip off the electrons entirely in order to create a plasma (a gas of ions and electrons). The electrons are super light compared to the ions so they shoot off, leaving behind a positively charged cloud of ions. These repel each other and also accelerate (though slower than the electrons) in a wave-like manner. They use these accelerators for similar applications as they use the more standard particle accelerators (like cyclotrons, synchrotrons, the LHC) but they generally have much lower energies. Applications would include nuclear/high energy particle physics, medical applications (beam therapy), nuclear reactions to create isotopes, etc.
kushm4sta
Profile Blog Joined July 2011
United States8878 Posts
June 02 2014 03:56 GMT
#5
how much can a physical chemist make?
OMGUS.net, kush sex blogs every friday night
urboss
Profile Joined September 2013
Austria1223 Posts
June 02 2014 09:42 GMT
#6
I don't know about physical chemistry, but the pay in science is usually decent enough.
Still nowhere near anything a doctor, lawyer or banker would make of course.

But hey, you get to do some awesome stuff in return.

The only problem is that the number of people that want to do science far exceeds the available positions. There are too many people that would rather forego earning any money than stop doing science. That's why most people end up working 80+ hours just to outcompete their peers.
So you better not be in it for the money, but rather because you actually enjoy doing the science.
Badjas
Profile Blog Joined October 2008
Netherlands2038 Posts
June 02 2014 09:43 GMT
#7
This blog hit the sweet spot where I can actually grasp what you mean and learn cool new stuff
Thanks!
I <3 the internet, I <3 you
kushm4sta
Profile Blog Joined July 2011
United States8878 Posts
June 02 2014 13:05 GMT
#8
i said physical chemistry, not science
OMGUS.net, kush sex blogs every friday night
Ideal26
Profile Blog Joined November 2013
United States185 Posts
June 02 2014 19:22 GMT
#9
On June 02 2014 12:56 kushm4sta wrote:
how much can a physical chemist make?


I couldn't tell you. I'm in physics (/engineering) and know very little about careers in the other sciences. It all depends on what you want to do. Professors can make decent money, but the process of getting up to tenure is painful. You'll have better luck going into industry if you don't want to fight a never-ending battle, but salaries there are super variable, as are job descriptions. It also depends on how many degrees you have.
urboss
Profile Joined September 2013
Austria1223 Posts
June 03 2014 07:28 GMT
#10
@ide, how about pasting these all into one thread called "Quantum Physics" and posting it in the general forum? Might get more attention there.
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